Tales from the Borderlands
35 Achievements
1,000
1-2h
Angry Eyes
Completed Episode 3
50
How to unlock the Angry Eyes achievement in Tales from the Borderlands - Definitive Guide
Story related, cannot be missed.
This trophy will unlock at the end of Episode 3: Catch a Ride. This episode will end with Rhys, Fiona and their friends being captured by Vallory. Gortys will tell Vallory that the final piece of her upgrade is located on Helios.
There really isn't much to explain for getting any of these achievements. All you need to do is complete the story. Nothing can be missed and no wrong decisions can be made, so you are able to tailor the experience to your preference. To get the full experience, you should investigate everything, or to speed through you can simply go to the proper objective.
The only thing worth noting is that you'll have to be quick in some of the action sequences, flicking the thumb stick in the proper direction, hovering over the proper item to select it, or mashing the proper button quickly. I never failed a sequence in my playthrough though, so it's really not that hard. The game will tell you what to do at all times with on-screen prompts, including when to use Rhys' echo eye ability.
You can find a playthrough with no commentary below.